本期封面文章
Article
Feng GONG, Yuhang JING, Rui XIAO*
Plasma-assisted ammonia synthesis under mild conditions for hydrogen and electricity storage: Mechanisms, pathways, and application prospects
——Front. Energy, 2024, 18(4): 418‒435
氨具有高储氢密度、清洁、高效、可再生等特点,是一种很有前途的零碳燃料。但传统的哈伯-博施(H-B)合成氨工艺需要高温高压,每年排放二氧化碳超过4.2亿吨,而且依赖于化石燃料。而介质阻挡放电(DBD)等离子体辅助合成氨则在低温、大气压下进行,利用高能电子激发的氮和氢自由基,为H-B工艺提供了潜在的替代方案。该方法可与可再生能源(如太阳能和风能)有效结合,实现环保、分布式、高效的氨生产。该综述对大气压低温DBD等离子体辅助合成氨技术进行了全面分析,涵盖了等离子体固氮的反应途径、机理和催化剂体系。根据目前的研究,综述中评估了 DBD 等离子体辅助氨合成技术的经济可行性,分析了现有的困境和挑战,并为非热等离子体氨工艺的未来提供了见解和建议。
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Review(封面文章)
论文标题:
Plasma-assisted ammonia synthesis under mild conditions for hydrogen and electricity storage: Mechanisms, pathways, and application prospects
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小提示:Frontiers in Energy为国产英文刊,不属于瑞士Frontiers系列。瑞士Frontiers系列相关期刊为Frontiers in Energy Research。