Green Energy & Environment（GEE）2024年第9卷第11期已正式出版。本期共收录文章11篇，其中research highlight 1篇，review article 3篇，research paper 7篇。欢迎大家阅读、下载和投稿！
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河北科技大学李发堂教授课题组——Constructing interfacial electric field and Zn vacancy modulated ohmic junctions ZnS/NiS for photocatalytic H2 evolution
该图整体色彩搭配以蓝色和金黄色为主，蓝色代表水和环保，金黄色突出纳米材料和科技的重要性。主体为中空纳米笼，这种设计通过宏观的视觉形象来代表微观的纳米结构，展现了科技与自然和谐共生的景象，形象表达了通过太阳能，将水光催化转化为绿色氢能的过程。右下角是ZnS/NiS空心纳米笼的分子模型，直观地表达了两者存在原子级界面。该研究利用费米能级移动策略设计欧姆接触，实现了ZnS/NiS界面上电子的高效传输，显著提高了光催化产氢性能。
图文目录
Research highlight page 1781-1783
Recyclable bio-based epoxy resin thermoset polymer from wood for circular economy
Bowen Zhang, Saravanakumar Elangovan, Zhuohua Sun*
https://doi.org/10.1016/j.gee.2024.08.007
Review article page 1784-1801
Application of ionic liquids in single-molecule junctions: Recent advances and prospects
Li Zhou1, Miao Zhang1, Yani Huo, Liping Bai, Suhang He, Jinying Wang*, Chuancheng Jia*, Xuefeng Guo*
Highlight the benefits of ionic liquids in single-molecule junctions (SMJs).
Illustrate the modulation mechanisms of ionic liquids in SMJs.
Summarize recent applications of ionic liquids in SMJs.
Propose potential future research topics about the integration of ionic liquids into SMJs.
https://doi.org/10.1016/j.gee.2024.01.003
Review article page 1802-1811
Melting points of ionic liquids: Review and evaluation
Zhengxing Dai, Lei Wang, Xiaohua Lu*, Xiaoyan Ji*
The melting points of the newest ILs are collected.
The factors of melting points are summarized and analyzed.
The predicted models of ILs melting points are reviewed and compared.
A framework for developing a quantitative model is proposed.
https://doi.org/10.1016/j.gee.2024.01.009
Review article page 1812-1821
Recent advances in water collection based on solar evaporation
Meijie Chen*, Shuang Li, Shuai Guo, Hongjie Yan, Swee Ching Tan*
Passive water collection rate is far less than its evaporation rate in the system.
Heat and mass transfer behaviors should be balanced on the evaporation side.
Subcooling, wettability, and geometry should be optimized to collect water.
Condensation & evaporation processes should be designed in a confined space.
https://doi.org/10.1016/j.gee.2024.05.005
Research paper page 1822-1834
Mechanochemical strategy assisted morphology recombination of COFs for promoted kinetics and LiPS transformation in Li–S batteries
Yunchen Ge, Yan Meng*, Lin Liu, Jianming Li, Xuechun Huang, Dan Xiao*
A Mechanochemical strategy of ball milling was applied to re-construct the morphology of COFs.
Different nano sizes of COFs were adapted to verify the reconstruction effect of the mechanical force.
DFT simulation illustrates the conversion active sites and deposition amount of Li2S in different morphologies of COF.
It provides a plan for the design and modification of the host COF materials in lithium-sulfur batteries.
https://doi.org/10.1016/j.gee.2023.03.005
Research paper page 1835-1846
Wood-derived freestanding integrated electrode with robust interface-coupling effect boosted bifunctionality for rechargeable zinc-air batteries
Benji Zhou1, Nengneng Xu1, Liangcai Wu*, Dongqing Cai*, Eileen H. Yu, Jinli Qiao*
Activation-doping assisted interface construction strategy is achieved in fabricating wood-derived integrated air electrode.
Interface coupling effect bestow superior catalytic properties on integrated air electrode.
The finely modulated electrode hydrophilicity ensures triple-phase boundary formation to accelerate mass transfer.
The obtained CoNiLDH@NPC exhibits remarkable bifunctional activity with potential gap of 0.70 V.
Zinc-air batteries based on CoNiLDH@NPC plate show superb performances in peak power density and cycling life.
https://doi.org/10.1016/j.gee.2023.12.002
Research paper page 1847-1856
Constructing interfacial electric field and Zn vacancy modulated ohmic junctions ZnS/NiS for photocatalytic H2 evolution
Yi-lei Li, Xu-jia Liu, Yun-biao Wang, Ying Liu, Rui-hong Liu, Hui-ying Mu, Ying-juan Hao, Xiao-jing Wang, Fa-tang Li*
Ohmic contact hollow VZn-ZnS/NiS nanocages is synthesized using ZIF-8 as a template.
The ohmic contact and Zn vacancies can cause electron rearrangement at the interface.
DFT indicates that charge rearrangement can reduce Gibbs free energy of hydrogen adsorption.
The activity of VZn-ZnS/NiS was 31.9 times higher than that of ZnS, reaching 10,636 μmol h−1 g−1.
https://doi.org/10.1016/j.gee.2023.12.007
Research paper page 1857-1865
Efficient nitric oxide capture and reduction on Ni-loaded CHA zeolites
Bin Yue, Jianhua Wang, Shanshan Liu*, Guangjun Wu, Bin Qin, Landong Li*
A promising sorbent Ni-CHA with NO uptakes up to 0.31 (lean) and 1.64 (rich) mmol/g.
Regeneration by NH3-purging-reduction at 673 K versus thermal desorption of 850 K.
NOx adsorption mechanism obtained through experimental and computational techniques.
https://doi.org/10.1016/j.gee.2023.12.005
Research paper page 1866-1877
Reusable salt-template strategy for synthesis of porous nitrogen-rich carbon boosts H2S selective oxidation
Xu Liu, Liang Shan, Xiaoxue Sun, Tianxin Wang, Zhongqing Liu*, Yuefeng Liu*
An environment-friendly and low-cost reused NaCl template strategy for synthesis of N-doped carbon.
The catalyst shows large specific surface areas, high pyridinic N content, and numerous structural defects.
The NC-10-800 catalyst exhibits superior H2S selective oxidation performance and outstanding stability.
The Lewis base site formed by pyridinic N acts as the active site to adsorb and dissociate H2S and O2.
https://doi.org/10.1016/j.gee.2024.01.005
Research paper page 1878-1890
Hybrid data-driven and physics-based modeling for viscosity prediction of ionic liquids
Jing Fan, Zhengxing Dai, Jian Cao, Liwen Mu, Xiaoyan Ji, Xiaohua Lu*
Systematic prediction errors in COSMO-RS model were revealed.
Establishing the quantitative relationship between residuals of the COSMO-RS model and quantum chemical descriptors.
The average absolute relative deviation was reduced from 52.45% to 1.54%.
Significant features on systematic deviations were captured.
https://doi.org/10.1016/j.gee.2024.01.007
Research paper page 1891-1900
Constructing lithiophilic sites–rich artificial solid electrolyte interphase to enable dendrite−free and corrosion−free lithium–sulfur batteries
Wei Lu1, Anshun Zhao1, Qiuxu Chen, Sihan Liu, Mingxi Yu, Zihao Wang, Ze Gao, Xue Zhao, Guiru Sun, Ming Feng*
MPAF-SEI consists of polyester polymer and LiF, Li–Al alloy lithiophilic sites.
Li symmetric cell runs stably for 3000 h under a capacity of 1 mA h cm-2.
Good electrochemical performances are achieved in Li–S cell under low N/P ratio of 4.
MPAF-SEI offers lithiophilic sites to reduce the nucleation overpotential of Li.
https://doi.org/10.1016/j.gee.2024.05.008
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影响因子
10.7
CiteScore
16.8
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