24年10月18日文献情报（11篇）

24年10月18日文献情报

1. 题目: Food waste biochar for sustainable agricultural use: Effects on soil enzymes, microbial community, lettuce, and earthworms

文章编号: N24101811
期刊: Chemosphere
作者: Akumuntu Athanasie, Eun Hea Jho, Seong-Jik Park, Jin-Kyung Hong
更新时间: 2024-10-18
摘要: This study investigates the effects of food waste biochar (FWB) on the biological properties of soil, including the microbial community structure, enzyme activities, lettuce growth, and earthworm ecotoxicity. This holistic assessment of various soil organisms was used to assess the potential of FWB as a soil amendment strategy. Pot experiments were carried out over a 28-d period using various FWB concentrations in soil (0–3% w/w). The presence of FWB enhanced the activity of alkaline phosphatase and beta-glucosidase in proportion to the FWB concentration. Similarly, the dehydrogenase activity after 28 d was positively correlated with the FWB concentration. Notably, the application of FWB improved the bacterial diversity in the soil, particularly among hydrocarbonoclastic bacteria, while also prompting a shift in the fungal community structure at the class level. Measures of lettuce growth, including total fresh weight, shoot length, and leaf number, also generally improved with the addition of FWB, particularly at higher concentrations. Importantly, FWB did not adversely affect the survival or weight of earthworms. Collectively, these findings suggest that FWB can enhance soil microbial enzyme activity and support plant growth-promoting rhizobacteria, potentially leading to increased crop yields. This highlights the potential of FWB as an eco-friendly soil amendment strategy.
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2. 题目: Advances in sustainable production and applications of nano-biochar

文章编号: N24101810
期刊: Science of the Total Environment
作者: Shristi Shefali Saraugi, Winny Routray
更新时间: 2024-10-18
摘要: Biochar is a carbonaceous material that can be amplified into nano-biochar (N-BC) using different physicochemical techniques. Contrary to bulk biochar, nano-biochar, and have better physicochemical characteristics, including a large specific surface area, pore properties, distinctive nanostructure, and high catalytic activity. The spotlight of this review is to contribute up-to-date information on the scaling up of biochar into nano-biochar through various sustainable techniques. This review paper is a compilation of research on nano-biochar from biochar including preparation, distinctive characteristics, and intended applications in the environmental and agricultural sectors, along with some other cutting-edge applications, which are all covered in detail in this review paper and also provides the knowledge gap that will be useful for future investigation and development.
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3. 题目: Dissolved organic matter-mediated adsorption behavior of benzophenones on functionalized covalent triazine frameworks

文章编号: N24101809
期刊: Chemical Engineering Journal
作者: Chao Zhu, Mingzheng Yang, Jiaxin Wu, Jun Wang, Qile Fang, Shuang Song, Baoliang Chen, Yi Shen
更新时间: 2024-10-18
摘要: Adsorption is a highly efficacious technique for the remediation of organic micropollutants (OMPs). However, the presence of dissolved organic matter (DOM) frequently impedes adsorbent process, with insufficient attention given to this influence. This study systematically evaluates the adsorption performance of covalent triazine frameworks (CTFs) functionalized with electron-donating or electron-withdrawing groups for benzophenones (BPs). The adsorption capacities of SO₃H-CTF, OH-CTF, and NH₂-CTF for BPs were 512.11 μmol/g, 1356.27 μmol/g, and 1421.85 μmol/g, respectively. The adsorption mechanism is predominantly governed by π-π electron donor–acceptor (EDA) interactions, supplemented by hydrogen bonding, particularly in hydroxyl-containing BPs, with electrostatic interactions being relatively negligible. Functionalization with − OH and − NH₂ groups increased the electron density in π-conjugated regions, enhancing BPs adsorption capacity, whereas − SO₃H modification, due to its electron-withdrawing nature, acted as a π electron acceptor. Importantly, the mediating role of humic acid (HA) in the adsorption process was investigated. The CTF-BPs-HA ternary system can either inhibit/enhance π-π EDA interactions between π-electron donor/acceptor and BPs by adsorbing onto the CTF materials. The HA-mediated system primarily affects the film diffusion stage, with minimal impact on pore diffusion and inner surface adsorption. The oxygenated functional groups in HA slightly enhanced hydrogen bonding within the adsorption system, with negligible influence on electrostatic interactions. In the presence of HA, the overall adsorption capacity of SO₃H-CTF decreased by 67.0 %, while that of OH-CTF and NH₂-CTF increased by 120.9 % and 55.3 %, respectively. This study elucidates the electronic behavior modifications of functionalized CTFs during BPs adsorption and underscores the significant role of HA in interaction mechanisms, providing theoretical guidance for the design of advanced adsorbents to enhance pollutant removal efficiency.
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4. 题目: The concentration of dissolved organic matter impacts the neurobehavior in zebrafish larvae exposed to cyclophosphamide

文章编号: N24101808
期刊: Environmental Science and Pollution Research
作者: Tianming Liu, Dongshen Shang, Weiqi Tian, Yindong Li, Rong Xie, Jianxing Zhao, Heru Dong
更新时间: 2024-10-18
摘要:

Dissolved organic matter (DOM) occurs ubiquitously in various water matrices and affects the chemical speciation and toxicity of emerging contaminants, such as cyclophosphamide (CP). However, the effects of CP in aquatic organisms with the presence of DOM have been relatively less addressed. In this study, zebrafish eggs < 4 h post fertilization (hpf) were exposed to CP (0 and 50 μg/L) and humic acid (HA, a main component of DOM, 0, 3, 10, and 30 mg-C/L) until 7 days post fertilization, and its toxicity was evaluated by behavioral approaches and transcription of nervous-related genes. An increase in swimming velocity and anxiety was noticed in zebrafish larvae exposed to CP. The related genes of neurotransmitter (drd1, mao, thp1b, and gad2), neurodevelopment (gli2b, nrd, and gfap), and neuroinflammation (thfα, casp3, and il-6) were upregulated by CP. In the presence of HA (3 mg-C/L), the behaviors and gene transcripts of zebrafish larvae were enhanced, while at 10 mg-C/L, they were mitigated. This study has demonstrated that DOM at low concentration increases the toxicity of CP and at high concentration alleviates its toxicity. This study highlights the importance of emerging contaminant exposure with the presence of DOM on their toxicities in aquatic organisms.

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5. 题目: Removal of cefuroxime from aqueous solution by biochars derived from antibiotic mycelial residue

文章编号: N24101807
期刊: Environmental Science and Pollution Research
作者: Xiaoli Ren, Yingfu Li, Tao Feng, Juan Lei, Lijun Cheng
更新时间: 2024-10-18
摘要:

In China, antibiotic mycelial residue is categorized as hazardous waste. To achieve the harmless and resourceful disposal of cephalosporin, three types of biochars from cephalosporin mycelia residues, namely non-activated carbon (BC1), ZnCl₂-activated carbon (BC2), and KOH-activated carbon (BC3), were respectively fabricated by high-temperature pyrolysis carbonization technology. These three kinds of biochars were characterized via iodine value, FTIR, and SEM, and the adsorption performance of the prepared biochars was investigated using cefuroxime (CXM) as the adsorption target. The results indicated that BC3 biochar possesses the most well-developed pores and the highest iodine value of 1367.41 mg/g; The most suitable dosage is 1.6 g/L, and the lower the pH, the more favorable the adsorption effect. The investigation of adsorption kinetics revealed that it conformed to the kinetic model of pseudo-second order, as well as the process of adsorption was governed by the chemical adsorption mechanism, the rate of adsorption was affected by the collective impact of the quantity of active sites present and the interaction strength between the CXM molecules and the biochar. The exploration of adsorption thermodynamics revealed that it aligned with the Langmuir model, the surface of biochar was relatively uniform, and the adsorption was mainly of low coverage; The calculation of thermodynamic parameters demonstrated that the adsorption was exothermic and spontaneous.

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6. 题目: Iron as a precursor of aggregation and vector of organic carbon to sediments in a boreal lake

文章编号: N24101806
期刊: Biogeochemistry
作者: Simon David Herzog, Viktoriia Mekelesh, Margarida Soares, Ulf Olsson, Per Persson, Emma Sofia Kritzberg
更新时间: 2024-10-18
摘要:

While organic matter (OM) interactions in the water column prevent iron (Fe) precipitation and sedimentation, Fe also acts as a precursor of aggregation and a vector of OM to sediments. This study aims to characterize Fe–OM interactions to understand the role of Fe in promoting aggregation and transport of OM. Samples of Fe and OM were collected from water, settling material, and sediment along a gradient starting from the inlet and continuing offshore within a boreal lake. Fe speciation was determined using X-ray absorption spectroscopy (XAS), and the chemical composition of OM was assessed using Diffuse reflectance infrared Fourier transform spectroscopy (DRIFT IR) and Nuclear magnetic resonance spectroscopy (NMR). The results show a decrease in Fe and OM concentrations in the water column with increasing distance from the inlet. Winter sampling revealed a shift in Fe speciation from dominance of organically complexed Fe to an increase in Fe(oxy)hydroxide, accompanied by a loss of aromatic and carboxylate function of OM. Summer sampling revealed no significant changes along the gradient, with Fe(oxy)hydroxide and carbohydrates dominating the water phase. Interestingly, settling particles and surface sediments were dominated by Fe(oxy)hydroxides and aliphatic OM. We propose that phototransformation may be an important process that influences the interaction between Fe and OM and, as a consequence, their fate along the spatial gradient. Our study suggests a photochemically induced loss of carboxylate groups, reflected by an increased carbohydrate-to-carboxylate ratio along the gradient, particularly in winter, and generally lower levels during summer. Loss of carboxylate function promotes the formation of Fe(oxy)hydroxides, which in turn, facilitates the aggregation and sinking of OM, particularly aliphatic components. These insights contribute to a broader understanding of carbon cycling and storage in lakes. Future studies should assess the significance of photochemical processes to OM burial and it how may change given trends in Fe and OM in northern regions.

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7. 题目: Enhanced anaerobic co-digestion of food waste and sewage sludge by co-application of biochar and nano-Fe3O4.

文章编号: N24101805
期刊: Journal of Environmental Management
作者: Liwen Luo, Roghayeh Karimirad, Jonathan W C Wong
更新时间: 2024-10-18
摘要: Conductive materials have been utilized to facilitate direct interspecies electron transfer (DIET) in anaerobic digestion (AD) to enhance methane production. However, the impact and efficacy of the co-application of biochar and nano-Fe3O4 have not been adequately elucidated, particularly their interaction on electron transfer efficiency. In this investigation, we examined the influence of simultaneously or independently adding biochar and nano-Fe3O4 to food waste (FW) and sewage sludge (SS) anaerobic co-digestion. A synergistic effect was observed under the co-application condition. Methane production reached 300.3 ± 19.8 mL/gCOD with the co-application of biochar and nano-Fe3O4, representing a 43.3%, 35.4%, and 5.4% increase compared to the sole Fe3O4, biochar, and nano-Fe3O4, respectively. Mechanistic analysis revealed that, in comparison to sole biochar and nano-Fe3O4, their co-occurrence significantly accelerated hydrolysis and acidogenesis, thereby enhancing the release of soluble organic components. Furthermore, the application of nano-Fe3O4 improved system stability and significantly promoted propionate degradation, maintaining a favorable condition for methane production. Additionally, the noteworthy increase in INT-ETS activity and cytochrome c concentration indicated that the co-application of biochar and nano-Fe3O4 stimulated electron transfer. Correspondingly, the activity of coenzyme F420, which indicates the performance of methanogenesis, exhibited a 2.44-fold increase compared to the control. This indicated that nano-Fe3O4 and biochar co-amendment can serve as a robust platform to strengthen DIET. This study provided a new insight regarding the application of biochar and nano-Fe3O4 in the AD system for strengthening electron transfer to promote methane production.
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8. 题目: Changes in Cd forms and Cd resistance genes in municipal sludge during coupled earthworm and biochar composting.

文章编号: N24101804
期刊: Ecotoxicology and Environmental Safety
作者: Zhimin Yu, Meng Zhou, Hongwei Zhang, Lei Yuan, Pin Lv, Limin Wang, Jizhou Zhang
更新时间: 2024-10-18
摘要: There is a close relationship between microbial activity and the bioavailability of heavy metals, and heavy metal resistance genes can affect the activity of heavy metals. To evaluate the effects of coupled earthworm and biochar composting on Cd forms and Cd resistance genes in sludge, the BCR continuous extraction method was applied to classify the Cd forms, and Cd resistance genes were quantitatively determined with heavy metal gene chip technology. The results showed that the changes in earthworm biomass during composting were sufficiently fitted by logistic models and that adding biochar effectively increased earthworm biomass. The coupled treatment of earthworms and biochar promoted the degradation of sludge. The coupled treatment of earthworms and biochar reduced the proportion of acid-extractable and reducible Cd relative to total Cd, increased the proportion of oxidized and residual Cd relative to total Cd, transformed Cd forms from active to inert, and reduced the gene copy number of Cd resistance genes (czcA, czcB, czcC, czcD, czcS, czrA, czrR, cadA, and zntA). czcB was identified as a key gene that affected acid-extractable Cd and residual Cd contents; czcA, czcB, czcD, and czcS were identified as key genes that affected the reducible Cd content; czrR and cadA were identified as key genes that affected the oxidized Cd content; and czcC was identified as a key gene that affected the total Cd content. Cd resistance genes could directly affect the Cd form or indirectly affect Cd form through their interactions with each other.
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9. 题目: The driving mechanism of diverse land use types on dissolved organic matter characteristics of typical urban streams from Wuhan city.

文章编号: N24101803
期刊: Journal of Environmental Management
作者: Hui Zhang, Zufan Liu, Jing Xu, Jun Yang, Xiang Zhang, Shiyong Tao
更新时间: 2024-10-18
摘要: Urban streams play a crucial role in water network connectivity, drainage and urban landscaping, and receive abundant allochthonous dissolved organic matter (DOM), which is derived from nature and human activities. However, the influence of diverse land use types on the spatiotemporal distribution and characteristics of DOM in typical urban streams is still not fully understood. Therefore, the water sample collection and data analysis campaign were carried out in Wuhan in summer and winter. By using parallel factor analysis (PARAFAC) model, two humic-like substances and one protein-like component were eventually identified, and the specific DOM charcteristics of urban streams in industrial area illustrated the impact of allochthonous DOM caused by anthropogenic activities on their properties. The characteristics of DOM presents spatiotemporal distribution differences, and the fluorescence intensity of DOM in summer was significantly higher than that in winter, mainly due to the variation of allochthonous input from precipitation and runoff. Significant differences of the DOM concentration and composition in urban streams under different vegetation coverage were found, indicating that extreme human disturbance and high vegetation coverage can both greatly change DOM characteristics in urban streams. Redundancy analysis (RDA) revealed an indirect driving effect of land use on DOM, and the influence was considerably stronger in summer. The partial least squares structural equation modelling (PLS-SEM) analysis showed that land use can directly affect DOM content of urban streams (-0.147), with anthropogenic land use playing a positive role and natural land use the reverse, and indirectly change DOM concentration by influencing DOM origin (0.128), nutrients (0.022) and heavy metals (0.021). Moreover, human social and economic structure in anthropogenic land use can affect DOM components and sources of urban streams. This study revealed the driving mechanism of land use impact on DOM characteristics and improve our understanding of DOM geochemical cycling in urban streams.
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10. 题目: The potential role of biochar in mitigating gaseous emissions from livestock waste - A mini-review.

文章编号: N24101802
期刊: Journal of Environmental Management
作者: Baitong Chen, Jacek A Koziel, Andrzej Bialowiec, Samuel C O'Brien
更新时间: 2024-10-18
摘要: The livestock industry plays a significant role in the economic well-being of many parts of the world with a host of environmental challenges. Key amongst them is the management of gaseous emissions emitted from livestock manure. Mitigation of gaseous emissions from livestock operations such as odor, odorous volatile organic compounds (VOCs), ammonia (NH3), hydrogen sulfide (H2S), and greenhouse gases (GHGs) have been of research interest for the last couple of decades. Biochar, a low-cost-value byproduct of biorenewable energy and thermochemical waste processing compared with syngas and bio-oil, has been actively researched as a potential surficial treatment of manure and emissions from stored or co-composted manure. Yet, the efficacy of biochar treatment differs, partly because biochar properties vary with feedstock and thermochemical processing conditions. To date, the results from laboratory-scale trials are encouraging, but a more focused effort is needed to bring this technology closer to farm-scale applications. Therefore, this review aims to summarize and highlight current research related to mitigating gaseous emissions from manure treated with biochar. Various types of biochar, and modes of biochar applications, e.g., manure additives and co-composting, dosage, and timing, are discussed in the context of targeted gas emissions mitigation. Gaps in knowledge remain, including demonstrated larger-scale mitigation performance and verifiable technoecomics. Standardization and certification of biochar properties suitable for specific environmental management applications are recommended. The potential synergy between mitigating emissions, improving manure quality, carbon, and nitrogen cycling in animal and crop production agriculture is found. Biochar can be a comprehensive solution to gaseous emissions while also upgrading manure as a high-quality additive that could improve the sustainability of animal and crop production systems.
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11. 题目: Iron-modified biochars and their aging reduce soil cadmium mobility and inhibit rice cadmium uptake by promoting soil iron redox cycling.

文章编号: N24101801
期刊: Journal of Environmental Management
作者: Tianren Si, Xin Chen, Rui Yuan, Siyu Pan, Yan Wang, Rongjun Bian, Xiaoyu Liu, Xuhui Zhang, Stephen Joseph, Lianqing Li, Genxing Pan
更新时间: 2024-10-18
摘要: Iron (Fe) modified biochar has been widely used for cadmium (Cd) contaminated soil remediation. However, the accompanying anions introduced during the modification process potentially affect the behavior of Cd in soil. In this study, we investigated the distinct Cd immobilization mechanisms by Fe2(SO4)3 modified biochar (FSBC) and Fe(NO3)3 modified biochar (FNBC) in a two-year pot experiment. Results showed that both FSBC and FNBC significantly reduced Cd concentrations in rice grains by 23%-42% and 30%-37% compared to pristine biochar (BC). Specifically, NFBC promoted the formation of amorphous Fe oxides by enhancing the NO3--reducing Fe(II) oxidation process, which significantly increased Fe/Mn oxide-bound Cd and decreased soil CaCl2-extractable Cd. For FSBC, the introduction of SO42- significantly promoted the formation of Fe plaques by enhancing the Fe(III) reduction process, which blocked the Cd transfer from the soil to the rice roots. More importantly, after two years of biochar application, an organo-mineral complex layer is formed on the biochar surface, which immobilized a large amount of Cd. The Cd immobilization on the surface of aged biochar could be due to the fixation by the secondary Fe oxides within the organo-mineral layer and the complexation by the surface functional groups. The result of laser ablation inductively coupled plasma mass spectrometry showed that the Cd content on aged FNBC and FSBC was 5.9 and 2.6 times higher than on aged BC. This might be attributed to the Fe-modified biochar's higher electron exchange capability (EEC), which promoted the development of organo-mineral complexes. Notably, the EEC of biochar was maintained during its aging process, which may keep the biochar surface active and facilitate continual Cd immobilization. This study revealed the complex mechanisms of soil Cd immobilization with Fe-modified biochar, providing new insights into sustainable biochar environmental remediation.
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